For the '66 300s, the 383 4bbl was standard, which came with a standard 3.23 axle ratio. SureGrip was optiona.. 2.76 was the 383 2bbl standard ratio, but was optional on the 383 4bbl. FWIW
As teh 383 4bbl is rated at 10.0CR, adding the 906 open chamber heads will lower the CR so that 93 pump octane works well, plus gets the better ports and larger exhaust valves. Something you can plan on later. For lower end torque, you usually want smaller hi-velocity ports for good cylinder filling at the lower rpms, NOT hogged-out ports that only flow well at .500" lift.
For a bit better cam, the '67 383 4bbl-spec cam was 256/260 degrees advertised duration, with the '68 "Road Runner" and '67 GTX cam being 268/284 degrees advertised duration. with about .450"+ lift. Which would equate to something in the 215 degrees @ .050" lift range.
I suspect the current Edelbrock PERFORMER intake for the 383 would be an updated version of the Edelbrock hi-rise aluminum intake which Chrysler sold in the old Direct Connetion parts program . . . WITH a factory Chrysler part number which made it legal for NHRA stock class drag racing, back then. A pahlpir of the B/RB HP exhaust manifolds would round out the combination, with a larger diameter dual exhaust with stock-type high-flow (possibly Steet Hemi spec mufflers). End result, an engine with good off-idle throttle response (NOT WOT off-idle, but once rolling) that will get decent fuel economy on highway trips AND be nice to drive, in general. A milder cam will help lower rpm response but the good dual exhaust will make it "a torque motor that will RPM".
On top of that low-height 4bbl intake is a 550cfm carb, so a better intake manifold with a more modern AFB or AVS2 would help a bit there.
IN the current state of affairs, even with the 383 and the good TorqueFlite, almost every 4cyl you mifght encounter can beat the car from a red light. Due to their lighter weight AND a "jillion-speed" automatic that has a 4.50 low gear in the trans. BUT the 383 with the 3.23 (or even a 2.76 has enough low-rpm torque to lay rubber, at least until the tires get traction, which is still respectable. The SG will make that a bit harder, though, as will wider rear tires!
So, get a stock-replacement cam for a '67+ 383 4bbl, with a new timing chain, plus a few maintenance issues on the engine (there are probably a few anyway). Get it running reliably, with new rubber fuel line sections from the fuel tank forward. And DRIVE it to learn more about how it feels. A set of good HD shocks is also good, along with new brake shoes, for good measure.
The car has definite possibilities! The interior is pretty nice, appearing to have been re-done previously, BUT sewn in teh factory pattern. So a little spiffing there would be good, but not necessary until later.
Enjoy!
CBODY67